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</html>";s:4:"text";s:5268:"Metallacarboranes are used in homogeneous catalysis, including hydrogenation, hydrosilylation, isomerization, hydrosilanolysis, phase transfer, burn rate modifiers in gun and rocket propellants, neutron capture therapy, medical imaging, processing of radioactive waste, analytical reagents, and as ceramic precursors. This page lists the known structurally characterised boranes according to structure type, closo-, nido-and arachno-and number of cluster vertices. hey are not However t necessary because each structure type has only one general formula, thus the formula gives the structure. 3 publications. The best known of these are elastomeric polycarboranylsiloxanes. The elucidation of the structure of diborane(6) led to the description of a new bond type, the three‐center bond, in which one electron pair is shared by three atomic centers. 5.03 Lecture 6 Polyhedral Boranes … endstream In chemical bonding: Boranes …form of closed frameworks (the closo-boranes), some looking like untidy birds’ nests (the nido-boranes), and some resembling spiderwebs (the arachno-boranes).Which type of structure is obtained correlates with the number of valence electrons in the molecule, and the correlation is expressed by Wade’s rules. Enter your email address below and we will send you your username, If the address matches an existing account you will receive an email with instructions to retrieve your username, This is an outdated version. Learn about our remote access options. 3. Your Mendeley pairing has expired. Heteroatoms generally exhibit a positional preference based on the order of the polyhedral vertex and the electron richness of the heteroatom relative to boron. These classifications apply equally well to boranes, heteroboranes, and their metalla analogues, and are intimately connected to a quantity known as the framework, or skeletal, electron count. A variety of boranes, heteroboranes, and metallaboranes undergo electrophilic substitution. Polyhedral boron hydrides and carboranes are used in neutron capture therapy of cancers, and as burn rate modifiers (accelerants) in gun and rocket propellant compositions. The term carborane is widely used in the American literature as a contraction of the IUPAC‐approved nomenclature carbaborane. By 1990 a great many nido metallaborane clusters has been characterized covering a wide range of sizes and polyhedral fragment geometries. New generations of tumor‐localizing boronated compounds are being developed. ChemInform Abstract: IS THE CLOSO, NIDO, OR ARACHNO CLASSIFICATION FOR BORANES A FUNCTION OF THE TOPOLOGICAL DESCRIPTION OF THE MOLECULE.. Systematization and structures of the boron hydrides. Type Nido- Arachno- Closo- Understandably many of the compounds have abbreviated common names. This article is cited by
Many of the deltahedra and deltahedral fragments have two or more nonequivalent vertices. There is a newer version of this article, I have read and accept the Wiley Online Library Terms and Conditions of Use,  10.1002/0471238961.0215181519030821.a01.pub2,  10.1002/0471238961.0215181519030821.a01, https://doi.org/10.1002/0471238961.0215181519030821.a01. Derivatives of 10B‐enriched closo‐borane anions and carboranes appear to be especially suitable. The important commercial tetrahydroborates are those of the alkali metals. Citations are the number of other articles citing this article, calculated by Crossref and updated daily. Nonequivalent vertices are recognized as having a different order; ie, a different number of nearest neighbor vertices within the framework. Please reconnect. Working off-campus? These classifications apply equally well to boranes, heteroboranes, and their metalla analogues, and are intimately connected to a quantity known as the framework, or skeletal, electron count. Trialkylamine and dialkylamine boranes, such as tri‐t‐butylamine borane and dimethylamine borane, are mainly used in electroless plating processes. Indeed, nearly all metals can be combined with polyborane hydride clusters to produce an apparently limitless variety of cluster compounds. Heteroboranes contain heteroelements classified as nonmetals. The Altmetric Attention Score is a quantitative measure of the attention that a research article has received online. The resulting hydridorhodacarboranes are quite robust and catalyze a number of reactions, including the isomerization and hydrogenation of olefins, the deuteration of B–H groups, and the hydrosilanolysis of alkenyl acetates. 51 0 obj From Nido to Arachno Boranes There is a steady progression of structures as one goes from a closo parent structure to successively more open nido and on to arachno boranes by the process of vertex subtraction. One such series is from closo (BH)2{6 to nido (BH) 5 H 4 (pentaborane-9), and on to arachno (BH) 4 H 6 (tetraborane-10). H‰œUÛnÛF}çWÌãn ®vygúdÇh» R‡mQXAAK”ņ"^¢:_ß™’’
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